Cavity-mediated thermal control of metal-to-insulator transition in 1T-TaS2
Cavity-mediated thermal control of metal-to-insulator transition in 1T-TaS2
Jarc, G.; Mathengattil, S. Y.; Montanaro, A.; Giusti, F.; Rigoni, E. M.; Sergo, R.; Fassioli, F.; Winnerl, S.; Zilio, S. D.; Mihailovic, D.; Prelovšek, P.; Eckstein, M.; Fausti, D.
Abstract
Placing quantum materials into optical cavities can provide a unique platform to control
quantum cooperative properties of matter, in the regimes of both weak and strong light-matter coupling. Here we show the first experimental evidence of the reversible touchless control of a metal-to-insulator phase transition in the charge density wave material 1T-TaS2 embedded in a tunable THz optical cavity. The switch between conductive and insulating behavior, which is obtained by mechanically tuning the distance between the cavity mirrors and their alignment, is related to a significant renormalization of the sample temperature. This suggests a Purcell-like scenario in which the spectral profile of the cavity modifies the energy exchange between the material and the external electromagnetic field. Our findings uncover a new path to control the thermodynamics and macroscopic transport properties of quantum materials by engineering their electromagnetic environment.
Keywords: metal-to-insulator transition; strong light-matter coupling; terahertz Fabry-Pérot cavity; phase transition
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Nature 622(2023)7983, 487-492
DOI: 10.1038/s41586-023-06596-2
Cited 11 times in Scopus
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Permalink: https://www.hzdr.de/publications/Publ-37545