Publikationsrepositorium - Helmholtz-Zentrum Dresden-Rossendorf

SrCu₂(BO₃)₂ is a quasi-two-dimensional spin system consisting of Cu²⁺ ions which form orthogonal spin-singlet dimers, also known as the Shastry-Sutherland lattice. This system has been studied extensively using a variety of techniques to probe the spin-triplet excitations, including recent magnetization measurements over 100 T. Spectroscopic techniques, such as nuclear magnetic resonance (NMR), can provide further insight into the spin-coupling mechanisms and excitations. We present ¹¹B NMR spectra measured in pulsed magnetic fields up to 54 T, and compare those with prior results obtained in static magnetic fields at 41 T. Herewith, we prove the feasibility and efficacy of this technique, yielding the capability for extended studies at highest magnetic fields up to the 100 T regime that determine the spin structure in the 1/3 magnetization plateau and beyond.